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Increased fluorescence of PbS quantum dots in photonic crystals by excitation enhancement

机译:通过激发增强增加光子晶体中pbs量子点的荧光

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摘要

We report on the enhanced fluorescence of lead sulfide quantum dots interacting with leaky modes of slab type silicon photonic crystals. The photonic crystal slabs were fabricated, supporting leaky modes in the near infrared wavelength range. Lead sulfite quantum dots which are resonant in the same spectral range were prepared in a thin layer above the slab. We selectively excited the leaky modes by tuning the wavelength and angle of incidence of the laser source and measured distinct resonances of enhanced fluorescence. By an appropriate experiment design, we ruled out directional light extraction effects and determined the impact of enhanced excitation. Three dimensional numerical simulations consistently explain the experimental findings by strong near field enhancements in the vicinity of the photonic crystal surface. Our study provides a basis for systematic tailoring of photonic crystals used in biological applications such as biosensing and single molecule detection, as well as quantum dot solar cells and spectral conversion applications
机译:我们报告了与平板型硅光子晶体的泄漏模式相互作用的硫化铅量子点增强的荧光。制造了光子晶体平板,在近红外波长范围内支持泄漏模式。在平板上方的薄层中制备了在相同光谱范围内谐振的亚硫酸铅量子点。我们通过调整激光源的波长和入射角度有选择地激发了泄漏模式,并测量了增强荧光的不同共振。通过适当的实验设计,我们排除了定向光提取的影响,并确定了增强激发的影响。三维数值模拟通过光子晶体表面附近的强近场增强一致地解释了实验结果。我们的研究为生物应用(例如生物传感和单分子检测)以及量子点太阳能电池和光谱转换应用中的光子晶体的系统定制提供了基础

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